The results of the asymmetric magneto-optical rotation in the magnetoplasmonic nanocomposite study are presented. The asymmetry is observed in spectra of magneto-optical rotation when a magneto-optical medium with a plasmonic subsystem is magnetized along or against the radiation wave vector. The asymmetry is observed as vertical displacement of a magneto-optical hysteresis loop too. Such asymmetry is detected in magnetoplasmonic nanocomposite, which consists of a magneto-optical layer of Bi substituted iron-garnet intercalated with a plasmonic subsystem of gold self-assembled nanoparticles. It is shown that the physical reason for the asymmetric magneto-optical rotation is the manifestation of the Cotton–Mouton birefringence effect when the normal magnetization of the sample to a radiation wave vector appears due to the magnetic component of the electromagnetic field of resonating nanoparticles. This effect is additive to the basic magneto-optical Faraday Effect.

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