DOI: 10.1177/01445987261468444 ISSN: 0144-5987

Recent advances in fabrication strategies for high-performance solid-state batteries: Overcoming interfacial challenges and enabling scalable, cost-effective manufacturing

Kannan Nithin K.V., Deepa Sundararajan, Ravi Samikannu, Satish G., Marimuthu C.N., Mohan S., Nyagong Santino David Ladu

The better energy density, improved safety, and longer cycle life of solid-state batteries (SSBs) make them a promising energy storage technology. Interfacial instability and manufacturing scalability still plague large-scale commercial adoption. Interface-engineered, Next Generation, Tailored, Energy-dense, Green, Reliable, Additive-manufactured, thermally stable, Economical (INTEGRATE) is a scalable fabrication strategy that leverages 3D printing, atomic layer deposition, and plasma-assisted processing. Our framework improves ion transport across the electrode–electrolyte interface, structural alignment during multilayer assembly, and mechanical compatibility under operational stress. Ionic conductivity of 0.025 S/cm at 338 K, 95% capacity retention after 250 cycles, 93% cycle-life retention over 500 cycles, $2.50 per cell fabrication cost, scalable production throughput of 260 units/hour, and 28% failure rate at 50 MPa are experimentally verified. The room-temperature ionic conductivity is 35% higher and the manufacturing cost is 25% lower than that of current methods. The INTEGRATE framework is a technically robust and economically scalable platform for high-performance SSB manufacturing, with strong potential for commercial deployment in electric vehicles, consumer electronics, and grid-scale energy storage systems, advancing next-generation sustainable energy technologies.

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