Observation of bandgaps in multilayer silicon nanoribbons
Zhicheng Gao, Dong Li, Hui Zhou, Jisong Gao, Xuegao Hu, Zhihao Cai, Qiaoxiao Zhao, Yudian Zhou, Peng Cheng, Kehui Wu, Lan Chen, Baojie FengOne-dimensional (1D) materials have attracted significant interest due to their unique quantum properties and potential applications in nanoscale devices. Pentagonal silicon nanoribbons (SiNRs), a prototypical 1D material, have been recently reported to host gapless Dirac fermions. However, for practical applications such as logic devices, the realization of a bandgap is highly desirable. In this work, we investigate the electronic structure of multilayer SiNRs grown on Ag(110) using angle-resolved photoemission spectroscopy. Our measurements reveal the emergence of a large bandgap at the Dirac point in these multilayer structures. Tight-binding model analyses suggest that the bandgap arises from the long-range periodicity along the nanoribbon chains. These findings demonstrate that multilayer SiNRs represent a novel phase of elemental silicon and provide a promising platform for engineering bandgaps in 1D materials, with potential applications in quantum and electronic devices.