Lattice engineering of thermally evaporated perovskite enables monolithically integrated micro-display
Jianfeng Ou, Zixi Shen, Shuwen Yan, Yuanwu Wu, Hongyi Xie, Xiang Zhang, Yannan Zhang, Jingshu Zhang, Zhengzheng Liu, Lei Li, Jianbo Wang, Juan Du, Luying Li, Jiajun Luo, Jiang TangPerovskite light-emitting diodes (PeLEDs) have recently demonstrated substantial potential for next-generation micro-displays due to their excellent efficiency and brightness. However, the best-performing PeLEDs typically suffer from low brightness and severe efficiency roll-off, as well as the considerable challenge of monolithic integration at pixel sizes down to 2 μm. Here, we present a lattice-engineering approach for thermally evaporated perovskites that simultaneously achieves high-performance PeLEDs and high-definition monolithic integration for perovskite micro-display applications. The lattice engineering achieved by in situ incorporation of FABr effectively suppresses Ruddlesden–Popper (RP) faults within nanocrystals and yields a uniform electric-field distribution, thereby reducing charge accumulation and suppressing Auger recombination. We further fabricated PeLEDs with a fully vacuum-deposited device architecture, demonstrating an external quantum efficiency (EQE) of 20.6% and high brightness levels exceeding 160,000 cd m −2 , with reduced efficiency roll-off. More importantly, through process and device optimizations, we achieved nanometer-scale conformal deposition on the surfaces of complementary metal-oxide-semiconductor (CMOS) driver pixel pits, thereby developing a perovskite micro-display with a resolution of 3,000 pixels per inch (PPI) capable of displaying vivid video. Our research paves the way for advancing micro-display technology.