DOI: 10.1021/acsaelm.6c01286 ISSN: 2637-6113

Flexible All-Fabric Pressure Sensors with Ultra-High Sensitivity and Wide Detection Range Fabricated via DIW-Printed AgNW Electrodes and AgNW/MXene Sensing Layers

Xinpeng Wang, Jiajun Huang, Zhijie Ye, Shihao Yang, Tingting Fu, Xianmou Guo, Bowen Li, Qi Yu, Yuehui Wang, Li Jingze

Abstract

Flexible wearable pressure sensors are crucial for personalized healthcare but suffer from inherent limitations: the “sensitivity-range trade-off” and the challenge of balancing sensing performance with textile breathability and comfort. To overcome these issues, a bilayer all-fabric piezoresistive sensor is developed by integrating direct ink writing and stepwise dip-coating to fabricate AgNW interdigital electrodes and an AgNW/MXene-coated sensing fabric, respectively. By leveraging the synergistic “point-line-surface” conductive architecture and the structural resilience of the knitted substrate, the sensor effectively resolves the conflict between high sensitivity and a wide detection range. It exhibits segmented high sensitivity: 1.29 × 108 (0–0.1 kPa), 1.19 × 107 (0.1–4 kPa), 9.19 × 105 (4–25 kPa), 4.15 × 105 (25–55 kPa), and 1.68 × 105 kPa–1 (55–120 kPa). It also boasts a broad working range up to 120 kPa, an ultra-low detection limit of 0.3 Pa, and rapid response/recovery times (18/39 ms). Practical validation confirms its versatility in full-range human motion monitoring from subtle physiological pulses to vigorous joint movements and advanced human–machine interaction, such as intelligent Morse code transmission and real-time mouse control. This work provides a versatile strategy for fabricating high-performance textile-based sensors, offering great potential for next-generation smart wearables and integrated health monitoring systems.

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