Achieving Large Uniaxial and Homogeneous Strain in Two‐Dimensional Materials

ABSTRACT

Strain is a powerful tool for tuning the electronic, magnetic, and topological properties of 2D materials ‐ particularly at high values of strain () where many electronic, magnetic, and structural transitions are predicted. However, most approaches to straining 2D materials are limited below 1.5%, with poor repeatability when cycling strain and low strain transfer upon cooling. Here, we report a high‐yield sample preparation and device strain platform that overcomes these limitations, enabling repeatable and reversible strain tuning up to the intrinsic strain‐to‐failure of the materials tested herein. We furthe r use this platform to controllably design uniform linear strain gradients, revealing a novel route for investigating flexoelectric and flexomagnetic phenomena. Using CrSBr as a standard for gauging strain, we demonstrate uniform uniaxial strain, up to 4%, with negligible slippage and linear strain gradients of up to 0.06%/. Our strain approach is applicable to a broad class of 2D materials, as validated by its performance for three different phases of transition metal dichalcogenides: 2H‐, 1‐ and ‐. In ‐, we show for the first time splitting of the and modes, starting at 2% strain, and record‐breaking strain up to 5.5% strain.