DOI: 10.1126/sciadv.aej9484 ISSN: 2375-2548

A continuous confinement-deconfinement transition in a triangular quantum magnet

Suguru Hosoi, Sejun Park, Michihiro Hirata, Minseong Lee, Adam P. Dioguardi, Joe D. Thompson, Filip Ronning, Allen O. Scheie, Kumpei Imamura, Kenichiro Hashimoto, Takasada Shibauchi, Bishnu P. Belbase, Arjun Unnikrishnan, Johannes Knolle, Arnab Banerjee, Yuji Matsuda

A continuous transition between phases hosting distinct excitations—bosonic magnons versus fermionic spinons—is a long-sought phenomenon in quantum magnetism, analogous to the confinement-deconfinement transition in quantum chromodynamics. We report evidence for such a transition in the triangular-lattice antiferromagnet thallium ytterbium disulfide. Antiferromagnetic order develops below T N  ≈ 0.53 kelvin. A c -axis field suppresses this order, driving the system into a gapless quantum spin liquid with a spinon Fermi surface above μ 0 H c ≈ 3   T , evidenced by a finite residual linear term in thermal conductivity, a Pauli-like susceptibility, and a temperature-independent nuclear magnetic resonance Knight shift. Approaching H c from above, the scattering rate of itinerant excitations is strongly enhanced, while their density of states shows no critical enhancement, atypical of conventional magnetic quantum criticality. These results point to a continuous confinement-deconfinement transition governed by fractionalized excitations beyond the Ginzburg-Landau paradigm.

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